Central Market has some really great, fresh, organic produce. If you're so inclined, you may also purchase produce by the case (and if you/your family can't eat it all yourself, you can split it with your raw/vegan friends) and save a bundle. They also have a lot of vegan options throughout the store, including quite a bit in the frozen foods selection. And, as Thoor said, lots of different tofu, even fried tofu cubes. I don't think I've seen that anywhere else. Also, you can find many ethnic items and seasonings that you can't really find too many other places.
Cons: A bit high priced, Need more vegan options in the deli, Lack of vegan cake (maybe that's a pro?)